I don't really have the best games, just roms, and I only have OoT and MM on Project64 (Unless I can get that WW torrent working...). Anyway, I find shipping and tragedy the most touching. So i'd say...
5. Marin tries to flirt to Link, but she's probably just a dream... sad.
4. Link leaves Saria, you could imagine both of them trying to fight back tears.
3. Link and Zelda after Byrne's defeat, cute, and comedic.
2. Byrne sacrifices himself, to make up for all of his actions... Noble.
1. Link and Zelda at the end of ST... Shipping evidence!
5. Marin tries to flirt to Link, but she's probably just a dream... sad.
4. Link leaves Saria, you could imagine both of them trying to fight back tears.
3. Link and Zelda after Byrne's defeat, cute, and comedic.
2. Byrne sacrifices himself, to make up for all of his actions... Noble.
1. Link and Zelda at the end of ST... Shipping evidence!